| Year | Category | Nominee(s) | Episode(s) | Result |
| 1967 | Outstanding Dramatic Series | Joseph Gantman and Bruce Geller | | Won |
| Outstanding Continued Performance by an Actor in a Leading Role in a Dramatic Series | Martin Landau | | Nominated |
| Outstanding Continued Performance by an Actress in a Leading Role in a Dramatic Series | Barbara Bain | | Won |
| Outstanding Writing Achievement in Drama | Bruce Geller | "Pilot" | Won |
| Outstanding Individual Achievements in Film and Sound Editing | Paul Krasny and Robert Watts | | Won |
| Individual Achievements in Music – Composition | Lalo Schifrin | | Nominated |
| 1968 | Outstanding Dramatic Series | Joseph Gantman | | Won |
| Outstanding Continued Performance by an Actor in a Leading Role in a Dramatic Series | Martin Landau | | Nominated |
| Outstanding Continued Performance by an Actress in a Leading Role in a Dramatic Series | Barbara Bain | | Won |
| Outstanding Directorial Achievement in Drama | Lee H. Katzin | "The Killing" | Nominated |
| Outstanding Writing Achievement in Drama | Allan Balter and William Read Woodfield | "The Seal" | Nominated |
| Outstanding Achievement in Art Direction and Scenic Design | Bill Ross | "Echo of Yesterday" | Nominated |
| Outstanding Achievement in Film Editing | David Wages | "The Photographer" | Nominated |
| Robert Watts | "The Traitor" | Nominated |
| Outstanding Achievement in Musical Composition | Lalo Schifrin | "The Seal" | Nominated |
| Special Classification of Individual Achievements | Joseph G. Sorokin | "The Survivors" | Nominated |
| 1969 | Outstanding Dramatic Series | Bruce Geller | | Nominated |
| Outstanding Dramatic Program | Alan Balter and William Read Woodfield | "The Execution" | Nominated |
| Outstanding Continued Performance by an Actor in a Leading Role in a Dramatic Series | Peter Graves | | Nominated |
| Martin Landau | | Nominated |
| Outstanding Continued Performance by an Actress in a Leading Role in a Dramatic Series | Barbara Bain | | Won |
| Outstanding Continued Performance by an Actor in a Supporting Role in a Series | Greg Morris | | Nominated |
| Outstanding Achievement in Art Direction and Scenic Design | Lucien Hafley and Bill Ross | "The Bunker" | Won |
| Outstanding Achievement in Musical Composition | Lalo Schifrin | "The Heir Apparent" | Nominated |
| 1970 | Outstanding Performance by an Actor in a Supporting Role in Drama | Greg Morris | | Nominated |
| Outstanding Achievement in Art Direction or Scenic Design – For a Dramatic Program or Feature Length Film, a Single Program of a Series or a Special Program | Lucien M. Hafley (set decorator) and Gibson Holley (art director) | | Nominated |
| Outstanding Achievement in Cinematography for Entertainment Programming – For a Series or a Single Program of a Series | Al Francis | | Nominated |
| Outstanding Achievement in Film Editing for Entertainment Programming – For a Series or a Single Program of a Series | Arthur David Hilton | | Nominated |
| Outstanding Achievement in Film Sound Mixing | Gordon L. Day and Dominick Gaffey | | Won |
| Outstanding Achievement in Any Area of Creative Technical Crafts | Jonnie Burke (Special Visual Effects) | | Nominated |
| 1971 | Outstanding Achievement in Film Sound Editing | Don Crosby, Douglas H. Grindstaff, Joe Kavigan, Chuck Perry and Frank White | | Nominated |
| Outstanding Achievement in Makeup | Robert Dawn | | Won |
| 1972 | Outstanding Performance by an Actor in a Supporting Role in Drama | Greg Morris | | Nominated |
| Outstanding Achievement in Art Direction or Scenic Design – For a Dramatic Program or Feature Length Film Made for Television, a Single Program of a Series or a Special Program | Lucien M. Hafley (set decorator) and Gibson Holley (art director) | | Nominated |
| 1973 | Outstanding Continued Performance by an Actress in a Leading Role (Drama Series – Continuing) | Lynda Day George | | Nominated |
| Outstanding Achievement in Art Direction or Scenic Design – For a Dramatic Program or Feature Length Film Made for Television, a Single Program of a Series or a Special Program | Lucien M. Hafley (set decorator) and Gibson Holley (art director) | | Nominated |
